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HtmlDocument.Images returns a collection of System.Windows.Forms.HtmlElement objects. To access attributes, such as ALT and SRC, that are not directly exposed by System.Windows.Forms.HtmlElement, use the HtmlElement.GetAttribute(string) method.
To add a new image to a document, either create a new IMG tag as a string, and assign it to the HtmlElement.InnerHtml property of an element previously added to the HTML DOM; or use the HtmlDocument.CreateElement(string) method, set its properties using HtmlElement.SetAttribute(string, string), and add it as a child of an existing element using HtmlElement.AppendChild(HtmlElement).